Osment expanded her repertoire into pop music and alternative/indie rock where she has recorded teen pop hits like "I Don't Think About It", "If I Didn't Have You" alongside her Hannah Montana co-star Mitchel Musso, and "Once Upon a Dream".Osment entered the world of music recording soundtracks for movie singles and Disney albums.Osment also had a voice-over role in a movie called Holidaze: The Christmas That Almost Didn't Happen, which also featured the voices of fellow Disney Channel stars Brenda Song and Dylan and Cole Sprouse. She also recorded the song "I Don't Think About It" for the movie's soundtrack.
The parade featured acts like Miley Cyrus and the High School Musical cast.
She and Musso performed a sketch based on a Hannah Montana episode. It earned her a Young Artist Award nomination in 2008 for "Best Performance in a TV Movie, Miniseries or Special Leading Young Actress".
After working in several television films in her childhood, she gained fame for co-starring as the character Gerti Giggles in Spy Kids 2: The Island of Lost Dreams and Spy Kids 3-D: Game Over.
She went on to co-star in the Emmy Award-nominated She also starred as Cassie in R. Stine's: The Haunting Hour Volume One: Don't Think About It and the Disney Channel Original Movie, Dadnapped as Melissa Morris.
She currently stars in the Freeform television series Young & Hungry as Gabi Diamond.
and Theresa Osment (née Seifert), an English teacher. Her father has appeared in various films, including her movie Soccer Mom, and her older brother is Academy Award-nominated actor Haley Joel Osment.
The series premiere scored record ratings for the Disney Channel with 5.4 million viewers, a response "beyond our wildest expectations", according to the president of Disney Channel Entertainment.
The show earned her a nomination for Young Artist Award in 2007 for best performance in a TV Series (Comedy or Drama).
According to an interview at the 2008 Grammys, she was writing some songs together with Eve 6.
In 2009 she signed with the Wind-up Records label and released "All the Way Up", the first single from her EP debut, All the Right Wrongs, released on October 26, 2009.
She also had a voice over role in a movie called Holidaze: The Christmas That Almost Didn't Happen.